Libra Compatibility with All 12 Zodiac Signs Best to WorstLibra love perfect horoscope signs are twins, water bearer, and aries. When it comes to matters of the heart, Libra seeks balance and compatibility above all else. The Twins can bring adventure and playfulness to the relationship, while The Water Bearer shares Libra's appreciation for wisdom and creativity. Aries, known for their intensity, can ignite a flame in Libra's soul. Libra and these signs create a balanced and satisfying relationship.